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Alexandre Ferreira's Molecular Modelling 2 Wiki Page!

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Ammonia

Ammonia Basic Information

A molecule of ammonia was constructed in Guassview and a Gaussian calculation was run, determining optimum geometry and bond lengths for the molecule, as well as molecular orbitals and vibrational data. identical optimization procedured were performed on Nitrogen, Hydrogen and Fluorine, which are shown below.

Name: Ammonia

Calculation Method: RB3LYP

Basis Set:6-31G(d,p)

Final Energy:-56.558

RMS Gradient:0.00000485

Point Group:C3V

N-H bond length: 1.02 A

The table below shows the results of the optimization. the table shows the force acting on the atoms of the molecule. force is the first derivative of potential energy, so the closer the force is to 0, the closer the potential energy is to a stationary point (a minimum)

         Item               Value     Threshold  Converged?
 Maximum Force            0.000004     0.000450     YES
 RMS     Force            0.000004     0.000300     YES
 Maximum Displacement     0.000072     0.001800     YES
 RMS     Displacement     0.000035     0.001200     YES
 Predicted change in Energy=-5.986276D-10

Optimized Structure

Log File For Ammonia

NH3 Log File

Interactive Model of molecule

test molecule

Vibrational Nodes

6 nodes expected

2 sets of degenerate modes (modes 2 and 3, and modes 5 and 6)

4 sets of degenerate nodes, 4 expected absorptions on spectra

Mode 1- Bending (umbrella node)
Modes 2 and 3- Bending
Mode 4- Stretching
Modes 5 and 6- Stretching

Ammonia Vibration Data Screenshot

Charge Distribution Data

Nitrogen Has charge of -1.125, each hydrogen has charge of 0.375. this is expected as nitrogen is more electronegative than hydrogen.

Nitrogen

Nitrogen Basic Information

Name: Nitrogen

Calculation Method: RB3LYP

Basis Set:6-31G(d,p)

Final Energy:-109.52

RMS Gradient:0.00000097

Point Group:DinfH

N-N bond length:1.106A

         Item               Value     Threshold  Converged?
 Maximum Force            0.000002     0.000450     YES
 RMS     Force            0.000002     0.000300     YES
 Maximum Displacement     0.000001     0.001800     YES
 RMS     Displacement     0.000001     0.001200     YES
 Predicted change in Energy=-8.782393D-13

Optimized Structure

Log File For Nitrogen

N2 Log File

Interactive Model of Molecule

test molecule

Vibrational Nodes

1 stretching mode expected, so 1 absorption reading in an IR spectra is expected

Nitrogen Vibrational Data Screenshot

Charge Distribution Data

Nitrogen is a neutral homonuclear diatomic molecule, so there is no dipole and there is a perfectly even charge distribution

Hydrogen

Hydrogen Basic Information

Name: Hydrogen

Calculation Method: RB3LYP

Basis Set:6-31G(d,p)

Final Energy:-1.18

RMS Gradient:0.00013

Point Group:DinfH

H-H bond length: 0.742

         Item               Value     Threshold  Converged?
 Maximum Force            0.000232     0.000450     YES
 RMS     Force            0.000232     0.000300     YES
 Maximum Displacement     0.000305     0.001800     YES
 RMS     Displacement     0.000431     0.001200     YES
 Predicted change in Energy=-7.091616D-08

Optimized Structure

Log File For Hydrogen

H2 Log File

Interactive Model of Molecule

test molecule

Vibrational Nodes

1 stretching mode expected, so 1 absorption reading in an IR spectra is expected

Hydrogen Vibrational Data Screenshot

Charge Distribution Data

Hydrogen is a neutral homonuclear diatomic molecule, so there is no dipole and there is a perfectly even charge distribution

Reaction Energy Calculation

2 molecules of nitrogen and 6 molecules of hydrogen react to create 2 molecules of ammonia. using these stoichiometric ratios and the energy of the molecules yielded by the optimization to calculated the change in energy of the reaction and thus determine whether the reactants or products are more stable.

Energy of hydrogen in au: -1.17853929

Energy of nitrogen in au: -109.52412868

Energy of ammonia in au: -56.55776873

Energy of Reactants: -113.05974655 au

Energy of Products: -113.11553746 au

Energy of reactants in kJ/mol:-296838.36

Energy of products in kJ/mol: -296984.84

Change in energy in kJ/mol:-146.48

Products (ammonia) is more stable than the reactants (nitrogen and hydrogen)

Analysis of a Fluorine Molecule

Fluorine Basic Information

Name: Fluorine

Calculation Method: RB3LYP

Basis Set:6-31G(d,p)

Final Energy:-199.50

RMS Gradient:0.00000070

Point Group:DinfH

F-F bond length:1.40

Item               Value     Threshold  Converged?
 Maximum Force            0.000001     0.000450     YES
 RMS     Force            0.000001     0.000300     YES
 Maximum Displacement     0.000001     0.001800     YES
 RMS     Displacement     0.000002     0.001200     YES
 Predicted change in Energy=-1.800054D-12

Optimized Structure

Log File For Fluorine

F2 Log File

Interactive Model of Molecule

test molecule

Vibrational Nodes

1 stretching mode expected, so 1 absorption reading in an IR spectra is expected

Fluorine Vibrational Data Screenshot

Charge Distribution Data

Fluorine is a neutral homonuclear diatomic molecule, so there is no dipole and there is a perfectly even charge distribution

Analysis of Select Molecular Orbitals

The orbital shown above is one of two identical π* antibonding orbitals formed by the 2p orbitals perpendicular to the internuclear axis (the 2p orbital paralel to the internuclear axis forms a σ orbital). these are important orbitals in fluorine as they an energy depth of -0.39au, the highest of any occupied orbital in fluorine, and are thus the Highest Occupied Molecular Orbitals (HOMO) in fluorine.

there are two of these orbitals because there are two 2p orbitals (2p_z and 2p_y, if the internuclear axis is defined as the x axis) which are perpendicular to the internuclear axis. the two orbitals are also perpendicular to each other (the three 2p orbitals are orthogonal to each other. the resulting molecular orbitals are degenerate and arranged perpendicularly to eachother, much like their constituent atomic orbitals.


The orbital shown above is the σ* antibonding orbital formed by the 2p orbitals parallel to the internuclear axis. this orbital is important in fluorine as it has an energy depth of -0.13au, the lowest of any unoccupied orbital, and thus is the lowest unoccupied molecular orbital (LUMO) in fluorine.

The orbital above is the σ bonding orbital formed by the 2s orbitals. this orbital has an energy depth of -1.34au, much lower than the orbitals discussed above.

The orbital above is the σ* antibonding orbital formed by the 2s orbitals. this orbital has an energy depth of -1.09au, much lower than the HOMO and LUMO orbitals discussed above.

The orbital above is the σ bonding orbital formed by the 1s orbitals. this orbital has an energy depth of -24.80au, much lower than all the orbitals discussed above, which range in energy depth from -0.13au to -1.34au). this characteristic of the orbital can be seen by how close it lies to the nuclei of the atoms relative to the other orbitals. unlike the orbitals above, this orbital has a principle quantum number of 1, which means that it does not contain valence electrons. the electrons in this orbital will never take part in any bonding.